High Temperature Electrochemical Energy Conversion and Storage Fundamentals and Applications 1st Edition by Yixiang Shi, Ningsheng Cai, Tianyu Cao, Jiujun Zhang 1351332019 9781351332019

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ISBN-10 :  1351332019 

ISBN-13 :  9781351332019

Author:   Yixiang Shi, Ningsheng Cai, Tianyu Cao, Jiujun Zhang 

As global demands for energy and lower carbon emissions rise, developing systems of energy conversion and storage becomes necessary. This book explores how Electrochemical Energy Storage and Conversion (EESC) devices are promising advanced power systems that can directly convert chemical energy in fuel into power, and thereby aid in proposing a solution to the global energy crisis. The book focuses on high-temperature electrochemical devices that have a wide variety of existing and potential applications, including the creation of fuel cells for power generation, production of high-purity hydrogen by electrolysis, high-purity oxygen by membrane separation, and various high-temperature batteries. High-Temperature Electrochemical Energy Conversion and Storage: Fundamentals and Applications provides a comprehensive view of the new technologies in high-temperature electrochemistry. Written in a clear and detailed manner, it is suitable for developers, researchers, or students of any level.

High-Temperature Electrochemical Energy Conversion and Storage: Fundamentals and Applications 1st Table of contents:

Chapter 1 Introduction to High-Temperature Electrochemical Energy Conversion and Storage
1.1 Introduction to Solid Oxide Fuel Cells
1.2 Introduction to Solid Oxide Electrolysis Cells
1.3 Molten Carbonate Fuel Cells
1.4 Introduction to High-Temperature Batteries
References
Chapter 2 Solid Oxide Fuel Cells
2.1 Introduction
2.2 Electrochemistry of SOFCs
2.3 Solid Oxide Fuel Cells Fueling with Syngas and Hydrocarbons
2.3.1 Hydrogen Electrochemical Oxidation
2.3.2 Carbon Monoxide Electrochemical Oxidation
2.3.3 SOFC Performance and Mechanisms with H2/CO Mixture Fuel
2.3.4 Hydrocarbon Electrochemical Oxidation
2.3.5 Carbon Deposition
2.4 Modeling and Simulation of Solid Oxide Fuel Cells
2.4.1 PEN Modeling of Solid Oxide Fuel Cells
2.4.2 Cell Unit Modeling of Solid Oxide Fuel Cells
2.4.3 Solid Oxide Fuel Cell Stack Modeling
2.5 Solid Oxide Fuel Cell System
2.5.1 Typical System Configurations
2.5.2 Fuel Processing for SOFC Systems
2.5.2.1 Internal Reforming
2.5.2.2 External Reforming
2.5.3 CO2 Capture in SOFC-Based Power Generation Systems
2.6 Summary
References
Chapter 3 Solid Oxide Electrolysis Cells
3.1 Introduction
3.2 Fundamentals of the Solid Oxide Electrolysis Cell
3.2.1 Basic Structures and Working Principles
3.2.2 Thermodynamics
3.2.3 Reaction Kinetics of SOECs
3.3 Reaction Mechanisms in Nickel-Patterned Electrodes
3.3.1 Carbon Deposition Mechanism
3.3.1.1 Distribution of Carbon Deposition
3.3.1.2 Structure Features of Deposited Carbon
3.3.2 Electrochemical Conversion Mechanisms of CO/CO2
3.3.2.1 Electrochemical Reaction Kinetics
3.3.2.2 Effects of Applied Voltage
3.3.2.3 Effects of Temperature
3.3.2.4 Effects of CO Partial Pressure
3.3.2.5 Effects of CO2 Partial Pressure
3.3.2.6 Reaction Mechanism Speculations for CO2 Electrolysis
3.4 Heterogeneous Chemistry and Electrochemistry of SOEC Porous Electrodes
3.4.1 Basic Performance
3.4.2 Analysis of Methane Production Pathways
3.4.3 Elementary Reaction Models and PEN Models
3.4.4 Effects of Key Parameters on the Negative Electrode Process
3.4.4.1 Sensitivity Analysis of Heterogeneous Elementary Reaction Rates
3.4.4.2 Effects of Applied Voltage
3.4.4.3 Effects of Negative Electrode Thickness
3.4.4.4 Active Zones for Heterogeneous Chemistry and Electrochemistry
3.4.4.5 Effects of Porosity and Particle Diameter
3.4.4.6 Effects of Ionic Conductivity
3.4.4.7 Effects of Gas Composition and Temperature
3.4.5 Coupling of Reactions and Transfer Processes in Positive Electrodes
3.4.6 Fuel-Assisted Electrolysis
3.5 Operating Condition Designs and Dynamic Behaviors in Tubular Cells
3.5.1 Experiment
3.5.2 Comprehensive Electrothermal Model for Tubular SOECs
3.5.2.1 Optimization of Conversion Ratio and Efficiency
3.5.2.2 Operating Condition Designs for Methane Production
3.5.2.3 Dynamic Operation Behaviors
3.6 High-Temperature Electrolysis Systems and Integration with Renewable/Fossil Energy Systems
3.6.1 System Integration and Typical Configurations
3.6.2 Novel Criteria for Renewable Power Storage Systems
3.6.3 Power Storage Strategies in Renewable Power Systems
3.7 Challenges and Outlooks
References
Chapter 4 Flame Fuel Cells
4.1 Introduction
4.2 Working Principles and Efficiency Analysis
4.3 Fuel-Rich Combustion
4.3.1 Types of Burners
4.3.1.1 McKenna Burner
4.3.1.2 Hencken Burner
4.3.1.3 Porous Combustors
4.4 FFC Performance
4.4.1 Electrochemical Performance
4.4.1.1 Effects of Equivalence Ratio
4.4.1.2 Effects of Gas Flow Rate
4.4.1.3 Effects of Burner–SOFC Distance
4.4.2 FFC Unit Configurations
4.5 Challenges in FFC
4.5.1 Thermal Shock Resistance
4.5.2 Carbon Deposition
4.5.2.1 Effects of Fuel Type
4.5.2.2 Effects of Materials
4.6 FFC Applications in CHP Systems
4.7 Summary
References
Chapter 5 Solid Oxide Direct Carbon Fuel Cell
5.1 Introduction
5.2 Thermodynamics of Carbon Conversion
5.2.1 Open Circuit Potential of DCFCs
5.2.2 Theoretical Efficiency of DCFCs
5.2.3 Practical Efficiency of DCFCs
5.3 DCFC Configurations
5.3.1 Solid Oxide DCFCs
5.3.2 Molten Media in DCFCs
5.3.2.1 Molten Carbonate in DCFCs
5.3.2.2 Liquid Metal in DCFC
5.4 Role of CO in Carbon Conversion
5.4.1 “CO Shuttle” Mechanism
5.4.2 Steam Gasification
5.4.3 Catalytic Gasification
5.4.4 Indirect Carbon Fuel Cell
5.5 Carbon Conversion in Molten Media
5.5.1 Wetting Conditions of Carbon by Molten Carbonate
5.5.2 Carbon Conversion Mechanisms in Molten Carbonate
5.5.3 Chemical and Electrochemical Reactions in Liquid Metal
5.5.3.1 Metal Oxidation in Liquid Metal Anodes
5.5.3.2 Carbon Conversion in Liquid Metal Anodes
5.6 Development of Carbon-Based Fuel Cell Stacks and Systems
5.6.1 Direct Carbon Fuel Cell Stacks and Associated Systems
5.6.2 Integrated Gasification Fuel Cell Systems
5.7 Chapter Summary
5.7.1 Technical Challenges of DCFCs
5.7.1.1 Current Collection of DCFCs
5.7.1.2 Molten Media Stability
5.7.1.3 Ash Content and Mineral Elements in Coal
5.7.2 Conclusions

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Tags: High Temperature, Electrochemical Energy, Storage, Fundamentals, Applications, Yixiang Shi, Ningsheng Cai, Tianyu Cao, Jiujun Zhang