Rational Design of Nanostructured Polymer Electrolytes and Solid Liquid Interphases for Lithium Batteries 1st edition by Snehashis Choudhury 3030289430 9783030289430

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ISBN-10 :  3030289430 

ISBN-13 :  9783030289430

Author:  Snehashis Choudhury 

This thesis makes significant advances in the design of electrolytes and interfaces in electrochemical cells that utilize reactive metals as anodes. Such cells are of contemporary interest because they offer substantially higher charge storage capacity than state-of-the-art lithium-ion battery technology. Batteries based on metallic anodes are currently considered impractical and unsafe because recharge of the anode causes physical and chemical instabilities that produce dendritic deposition of the metal leading to catastrophic failure via thermal runaway. This thesis utilizes a combination of chemical synthesis, physical & electrochemical analysis, and materials theory to investigate structure, ion transport properties, and electrochemical behaviors of hybrid electrolytes and interfacial phases designed to prevent such instabilities. In particular, it demonstrates that relatively low-modulus electrolytes composed of cross-linked networks of polymer-grafted nanoparticles stabilize electrodeposition of reactive metals by multiple processes, including screening electrode electrolyte interactions at electrochemical interfaces and by regulating ion transport in tortuous nanopores. This discovery is significant because it overturns a longstanding perception in the field of nanoparticle-polymer hybrid electrolytes that only solid electrolytes with mechanical modulus higher than that of the metal electrode are able to stabilize electrodeposition of reactive metals.

Rational Design of Nanostructured Polymer Electrolytes and Solid Liquid Interphases for Lithium Batteries 1st Table of contents:

1. Introduction
2. Hybrid Hairy Nanoparticle Electrolytes Stabilize Lithium Metal Batteries
3. A Highly Reversible Room-Temperature Lithium Metal Battery Based on Cross-Linked Hairy Nanoparticles
4. Confining Electrodeposition of Metals in Structured Electrolytes
5. Lithium Fluoride Additives for Stable Cycling of Lithium Batteries at High Current Densities
6. Designing Solid-Liquid Interphases for Sodium Batteries
7. Electroless Formation of Hybrid Lithium Anodes for High Interfacial Ion Transport
8. Designer Interphases for the Lithium-Oxygen Electrochemical Cell
9. Soft Colloidal Glasses as Solid-State Electrolytes
10. Solid Polymer Interphases for Lithium Metal Batteries
11. Stabilizing Polymer Electrolytes in High-Voltage Lithium Batteries

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Tags: Rational Design, Nanostructured Polymer, Electrolytes, Solid Liquid Interphases, Lithium Batteries, Snehashis Choudhury